文部科学省 科学研究費補助金 学術変革領域研究(B)2021年度~2023年度

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表面水素工学 スピルオーバー水素の活用と量子トンネル効果の検証

研究成果

 論文

[A05班] Yoyo Hinuma, 「Systematic derivation of maximally orthogonalized supercells」Science and Technology of Advanced Materials: Methods, 2022, 2, 266-279. (DOI: 10.1080/27660400.2022.2093094)

[A05班] Yoyo Hinuma, 「Modeling interfaces of fluorite-structure compounds using slab charge distribution」Science and Technology of Advanced Materials: Methods, 2022, 2, 392-401. (DOI: 10.1080/27660400.2022.2126739)

[A03班] Chunmei Tang, Ning Wang, Ruijie Zhu, Sho Kitano, Hiroki Habazaki and Yoshitaka Aoki, 「Design of Anode Functional Layers for Protonic Solid Oxide Electrolysis Cells」J. Mater. Chem. A, 2022, 10, 15719-15730. (DOI: 10.1039/d2ta02760g)

[A03班Hajime Toriumi, SeongWoo Jeong, Sho Kitano, Hiroki Habazaki, and Yoshitaka Aoki, 「Enhanced Performance of Protonic Solid Oxide Steam Electrolysis Cell of Zr-Rich Side BaZr_0.6 Ce_0.2 Y_0.2 O_3−δ Electrolyte with an Anode Functional Layer」ACS Omega, 2022, 7, 9944-9950. (DOI: 10.1021/acsomega.2c00569)

[A01班, A05班] Shun Kazuki, Kohsuke Mori, Shinya Masuda, Naoki Hashimoto, Yoyo Hinuma, Hisayoshi Kobayashi, and Hiromi Yamashita, 「Revealing Hydrogen Spillover Pathways in Reducible Metal Oxide」, Chemical Science, 2022, 13, 8137-8147. (DOI: 10.1039/d2sc00871h)

[A01班] 森 浩亮, 橋下直樹, 山下弘巳, 「水素スピルオーバーを利用した5元系ハイエントロピー合金ナノ粒子の調製と触媒機能」触媒, 2022, 64, 79-85.

[A02班] Moe Takabatake, Ken Motokura, 「Montmorillonite-based Heterogeneous Catalysts for Efficient Organic Reactions」, Nano Express, 2022, 3, 014004. (DOI: org/10.1088/2632-959X/ac5ac3)

[A05班, A01班] Yoyo Hinuma, Kohsuke  Mori, 「Geometrical Determination of Surface Atom Diffusion Paths」, Materials Transactions, 2022, 63, 720-725. (DOI: https://doi.org/10.2320/matertrans.MT-M2021225)

[A01班] 森 浩亮, 「壊れにくい金属ナノ粒子の低温・簡便な合成に成功 ―高活性・高温強度・高耐久性を兼ね備えた次世代触媒として期待―」プレスリリース

[A01班] Kohsuke Mori, Naoki Hashimoto, Naoto Kamiuchi, Hideto Yoshida, Hisayoshi Kobayashi, Hiromi Yamashita, 「Hydrogen Spillover-driven Synthesis of High Entropy Alloy Nanoparticles as a Robust Catalyst for CO2 Hydrogenation」, Nature Communications, 2021, 12, 3884–3893. (DOI: https://doi.org/10.1038/s41467-021-24228-z)

招待講演

[A01班] 森 浩亮,「カーボンニュートラル社会構築を目指した金属有機ハイブリッド触媒の開発」, 産研 次世代材料セミナー<金属有機融合材料に関する最新研究紹介と社会実装に向けた将来展望>, Aug. 18, 2022.

[A01班] 森 浩亮,「 次世代合金ナノ粒子触媒開発のための理論計算の活用」【Daikin Webinar】カーボンニュートラル社会へ向けたCO2分解・回収・再利用 研究事例のご紹介, Aug. 4, 2022.

[A01班] Kohsuke Mori, 「Nanocatalyst Engineering for CO2 Hydrogenation to Formic Acid as a Promising Hydrogen Storage Material」, ICEC2022, Aug. 1, 2022.

[A01班] Kohsuke Mori, 「Controlled Release of Hydrogen Isotope Compounds in the Heterogeneously-catalyzed Formic Acid Dehydrogenation」, Taipei International Conference on Catalysis (TICC-2022), July 21, 2022.

[A02班] 本倉 健, 「Development of Supported Catalyst Systems for Highly Efficient/Challenging Organic Reactions」, International Conference on State-of-the Art Catalysis and Surface/Interface Science for Sustainable Society - 11th Iwasawa Conference, Mar. 11, 2022.

[A02班] 本倉 健, 「固体酸触媒と金属錯体・金属ナノ粒子の協奏効果による反応加速」, 令和3年度 触媒学会東日本支部講演会 (第31回 規則性多孔体セミナー)―固体酸触媒能の究明に向けて―, Jan. 21, 2022.

[A02班] Ken Motokura, 「Synergistic Catalysis of Supported Metal Catalysts for Fine Chemicals Synthesis」, The 2nd International Electronic Conference on Catalysis Sciences—A Celebration of Catalysts 10th Anniversary, Oct. 27, 2021.

[A01班] Kohsuke Mori, 「Nanocatalyst Engineering for Formic acid/CO2-mediated Chemical Hydrogen Delivery/Storage」, 1st Japan-China Symposium on Catalysis (1stJCSC), Oct. 10, 2021.

[A02班] Ken Motokura, 「Homogeneous and Heterogeneous Catalysts for CO2 Conversion Reactions」, The 3rd Japan-China Forum on Clean Energy, Sept. 26, 2021.

[A02班] 本倉 健, 「同一固体表面および触媒粒子間での協奏的触媒作用によるファインケミカルズ合成"」 第128回触媒討論会, オンライン, Sept. 1, 2021.

[A04班] Takashi U. Ito, 「mu+SR as a Potential Tool for Depth-resolved Detection of Oxygen Vacancies in Perovskite Oxides」, Materials Research Meeting 2021, Yokohama, Dec. 16, 2021.

[A01班] Kohsuke Mori, 「Nanocatalyst Engineering for CO2 Hydrogenation to Formic Acid as a Promising Hydrogen Storage Material」, 17th Japan-Taiwan Joint Symposium on Catalysis, Online, Dec. 4, 2021.

[A04班] Takashi U. Ito, 「Positive Muons in SrTiO3: Electronic Structure of the Hydrogen-Like Defects and Their Potential Use in Depth-Resolved Detection of Oxygen Vacancies」, The 9th International Symposium on Surface Science, Online, Nov. 30, 2021.

 

受賞

[A01班] Naoki Hashimoto, Kohsuke Mori, Hiromi Yamashita, Development of novel synthesis of high entropy alloy nanoparticles as durable catalysts for CO2 hydrogenation」,  ICEC Poster Award, Aug. 2, 2022.

[A01班] Naoki Hashimoto, Kohsuke Mori, Hiromi Yamashita, 「Synthesis of High-Entropy Alloy Nanoparticles by the Assist of Hydrogen Spillover as a Robust Catalyst for CO2 Hydrogenation」,  TOCAT9 Poster Prize, July 27, 2022.

[A01班] Naoki Hashimoto, Kohsuke Mori, Hiromi Yamashita, 「Synthesis of High Entropy Alloy Nanoparticles Assisted by Hydrogen Spillover of TiO2 Support and Investigaion of Catalytic Property」,  18th Japan-Korea Symposium on Catalysis, Best Presentation Award, Nov. 23-25, 2021.

[A02班] Moe Takabatake, Ken Motokura, 「Dehydrogenative coupling of alkane and benzene accelerated by interparticle hydrogen transfer』, 18th Japan-Korea Symposium on Catalysis, Best Poster Award, Nov. 23-25, 2021.

[A02班] 佐藤 吏沙⼦, 本倉 健, 「Mg-Al ハイドロタルサイトによる⽔素移動・環化反応を経由するキノリン誘導体のワンポット合成」第11回CSJ化学フェスタ2021, 優秀ポスター発表賞, Dec. 1, 2021.

[A02班] 高畠 萌, 本倉 健, 「担持白金触媒と固体酸触媒の混合系によるアルカンを用いるベンゼンのアルキル化反応」第11回CSJ化学フェスタ2021, 優秀ポスター発表賞, Dec. 1, 2021.

[A02班] 高畠 萌, 本倉 健, 「粒子間水素移動によって加速されるアルカンとベンゼンの脱水素カップリング反応」, 触媒学会若手会第41回 夏の研修会, ポスター発表優秀賞, Aug. 5, 2021.